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Overview

Our research is concerned with the development of materials and methods for use in radiation dosimetry using luminescence techniques. Our major interests are in the development of Thermoluminescence (TL) and Optically Stimulated Luminescence (OSL) in radiation dosimetry. These methods have applications in environmental dosimetry, personal dosimetry, high dose dosimetry, medical dosimetry, retrospective (accident) dosimetry, space dosimetry and archaeological dating. 

(a) Dosimetry:
Most recent interest has concerned the the development of anion-deficient Al2O3 doped with carbon as a sensitive OSL dosimeter using visible light to stimulate the emission. Our recent work has resulted in the development of a Pulsed OSL technique (POSL) dosimetric readout method. The technology is licensed by Landauer Inc. and in their dosimeter, sold under the trade name LuxelTM.

A second major project within the lab is the development of Al2O3 fiber optic probes for use in radiotherapy dosimetry. The goal is to develop a dosimeter probe which is small enough to place within the body for near-real-time measurement of the absorbed dose during radiotherpay treatment for cancer. (Sponsored by the Oklahoma Center for the Advancement of Science, and Landauer Inc.)

Another major interest of the lab is in the development of novel UV dosimetry techniques. Current work has led to the development of a dosimeter based on OSL from Al2O3:C for the assessment of UVB exposure. Projects testing the UVB response of other dosimetry materials are also underway.(Sponsored by the State of Oklahoma.)

A recent new interest is the development of luminescence dosimetry techniques for astronauts in Low Earth Orbit.  Both OSL and TL of a variety of materials are being examined for potential applications in space, where the complex radiation environment presents a challenge for conventional dosimetry methods and procedures. This project is part of the group's activities within the Arkansas-Oklahoma Center for Space and Planetary Sciences (see below). (Sponsored by NASA and NSF.)

(b) Dating:
Techniques in luminescence dating which are of interest include OSL and TL single aliqout and single grain procedures on quartz and feldspars. Applications of interest include the dating of eolian and fluvial Holocene sand dunes in central Oklahoma, and the potential for modification of these methods for dating sediments trapped within ice cores. (Sponsored by the State of Oklahoma.)

We are developing objective ways to analyze large statistical data sets obtained from Single Aliquot Regeneration (SAR) methods as applied to quartz and feldspar. Applications of the methods have been demonstrated in Holocene sands in Oklahoma and South Australia. (Sponsored by NSF and by the State of Oklahoma.)

An exciting project is the development of instrumentation and techniques for the potential application of luminescence dating on the surface of Mars, using robotic in-situ instrumentation. We are collaborating with the Jet Propulsion Laboratory, other NASA Centers, and the private sector to develop the necessary instrumentation, while at the same time developing the techniques required to date martian surface sediments using instrumentation of this type. (Sponsored by NSF and  by the State of Oklahoma.) 

(c) Theoretical Developments:
Our research interests also include numerical modeling of the processes of TL and OSL production. Numerical analysis of the rate equations describing the production of TL and OSL yield significant insight into the dynamics of the luminescence mechanisms. These techniques have been applied with success to understanding the TL and OSL properties of quartz (SiO2) and Al2O3, especially as applied to their use in dosimetry and archaeological dating. (Sponsored by the State of Oklahoma.)
 

Major Equipment

Major OSL and TL equipment includes three Risoe DA-15 TL/OSL systems, with OSL stimulation sources of green diodes, blue diodes, broad-band visible, IR diodes and IR lasers.  Irradiation facilities included with the systems consist of beta and alpha sources.

For other OSL-related investigation we have a 2nd-harmonic Nd:YAG pulsed laser, an Ar-ion laser (6 W, all lines) with UV optics, and a 10 ns pulsed nitrogen laser. We have a Jobin-Yvon spectrofluormeter for TL, OSL and photoluminescence spectral measurements. The laboratory is also generously equipped with various light sources, spectrometers, light detection systems and electronic test equipment. Photoconductivity; thermally stimulated conductivity (TSC)  and  additional thermoluminescence (TL) facilities consist of two computer-controlled 4 K-to-room temperature systems, each capable of measuring currents as low as 10-15 A. These systems allow  simultaneous TSC and TL measurements. A high temperature TL system is also available. A photoconductivity system, consisting of an Oxford Instruments continuous flow cryostat is also available. Perkin-Elmer Model 330 and Varian Cary 5 spectrophotometers are available for routine absorption measurements in the near-ir-vis-uv ranges. A Nicolet FTIR spectrophotometer is also available for absorption measurements in the infrared.. Radiation sources consist of 60Co and 137Cs gammasources, a 90Sr/90Y beta source, a 244Cm alpha source, a 40kVp x-ray source, and a Pu:Be neutron source.
 

Address

Optically / Thermally Stimulated Laboratory
Department of Physics
145 Physical Sciences
Oklahoma State University
Stillwater, OK 74078-3072
 
Telephone: +1 405 744 6455
Fax: +1 405 744 6811
For more information please contact: S.W.S. McKeever
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Last modified November 18, 2004